RegistryKey skms = SoftwareKey.OpenSubKey(RegistryKeyName, true);
The second parameter should be set to true if you need write access to the key.
On 64-bit system, you can try this (if you are using .Net 4):
private readonly RegistryKey SoftwareKey = RegistryKey.OpenBaseKey(RegistryHive.LocalMachine, RegistryView.Registry64). OpenSubKey("SOFTWARE");
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