maxReceivedMessageSize and maxBufferSize in app.config

You need to do that on your binding, but you’ll need to do it on both Client and Server. Something like:

<system.serviceModel>
    <bindings>
        <basicHttpBinding>
            <binding maxBufferSize="64000000" maxReceivedMessageSize="64000000" />
        </basicHttpBinding>
    </bindings>
</system.serviceModel>

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